|本期目录/Table of Contents|

[1]李 欢,张沁瑞*,闫广新,等.2005~2018年北京平原区土壤汞时空特征及其影响因素[J].地球科学与环境学报,2023,45(01):93-103.[doi:10.19814/j.jese.2022.10045]
 LI Huan,ZHANG Qin-rui*,YAN Guang-xin,et al.Tempo-spatial Characteristics of Soil Mercury in Beijing Plain, China from 2005 to 2018 and Their Influence Factors[J].Journal of Earth Sciences and Environment,2023,45(01):93-103.[doi:10.19814/j.jese.2022.10045]
点击复制

2005~2018年北京平原区土壤汞时空特征及其影响因素(PDF)
分享到:

《地球科学与环境学报》[ISSN:1672-6561/CN:61-1423/P]

卷:
第45卷
期数:
2023年第01期
页码:
93-103
栏目:
环境与可持续发展
出版日期:
2023-01-15

文章信息/Info

Title:
Tempo-spatial Characteristics of Soil Mercury in Beijing Plain, China from 2005 to 2018 and Their Influence Factors
文章编号:
1672-6561(2023)01-0093-11
作者:
李 欢张沁瑞*闫广新黄 勇
(北京市生态地质研究所,北京 100120)
Author(s):
LI Huan ZHANG Qin-rui* YAN Guang-xin HUANG Yong
(Beijing Institute of Ecological Geology, Beijing 100120, China)
关键词:
土壤汞 时空特征 重金属 正态性检验 半变异函数 影响因素 北京
Keywords:
soil mercury tempo-spatial characteristic heavy metal normality test semi-variance influence factor Beijing
分类号:
X53
DOI:
10.19814/j.jese.2022.10045
文献标志码:
A
摘要:
为了解北京平原区土壤汞的分布特征及变化规律,采样测定了2005、2015、2018年的土壤汞含量,获取了270条实验测试数据。采用定量与定性分析相结合的方式,阐述了土壤汞的时间和空间变化特征,并对影响土壤汞时空特征的因素进行了探讨。结果表明:北京平原区土壤汞含量整体呈下降趋势,2005~2015年由0.093×10-6下降至0.064×10-6,到2018年下降至0.058×10-6,逐渐接近甚至低于北京市土壤背景值; 土壤汞的块基比为28.2%~29.9%,空间自相关性中等,空间结构受结构性因素和随机性因素的共同影响,在空间分布上呈现出“城区含量高、郊区含量低”的特点; 由于外界输入土壤内部的含汞物质大幅度降低(输入减少),以及土壤中的汞通过排放、转化、吸收等方式不断流失(输出持续),造成2005~2018年土壤汞含量不断下降; 工业生产、人类生活、城市建设历史等人为源加剧了城区土壤汞的富集,反映了随机性因素的影响; 水系流域、土壤质地等自然源造成土壤汞分布的局部性差异,反映了结构性因素的影响。
Abstract:
In order to understand the distribution characteristics and variations of soil mercury in Beijing plain, the contents of soil mercury in 2005, 2015 and 2018 were sampled and measured, and 270 analytical data were obtained. A combination of quantitative and qualitative analysis was used to explore the tempo-spatial variation of soil mercury, and to analyze the influence factors affecting the tempo-spatial characteristics of soil mercury. The results show that the contents of soil mercury in Beijing plain decrease from 0.093×10-6 in 2005 to 0.064×10-6 in 2015, and to 0.058×10-6 in 2018, which is close to or even lower than the soil background value in Beijing; the block-base ratios of soil mercury are 28.2%-29.9%, indicating that the spatial autocorrelation of soil mercury is moderate, and the spatial structure is affected by both structural and random factors; the spatial distribution of soil mercury in Beijing plain is characterized by “high content in urban areas, and low content in suburbs”; the mercury-containing substances imported from the outside into the soil are greatly reduced(input reduces), and the mercury in the soil is continuously lost through discharge, transformation and absorption(output continues), resulting in the continuous decline of the contents of soil mercury from 2005 to 2018; industrial production, human life, urban construction history and other human factors can aggravate the enrichment of mercury in urban soil, reflecting the impact of random factors; natural factors such as drainage basin and soil texture cause local differences in the distribution of soil mercury, reflecting the impact of structural factors.

参考文献/References:

[1] 董丽君,张展华,张 彤.土壤环境汞污染现状及其影响因素研究进展[J].地球与环境,2022,50(3):397-414.
DONG Li-jun,ZHANG Zhan-hua,ZHANG Tong.Mercury Pollution in Soil Environment:Current Status and Its Influencing Factors[J].Earth and Environment,2022,50(3):397-414.
[2] 李洪奎,李逸凡.山东日照地区土壤重金属环境质量评价[J].地球科学与环境学报,2018,40(4):473-486.
LI Hong-kui,LI Yi-fan.Environmental Quality Eva-luation of Soil Heavy Metals in Rizhao Area of Shandong,China[J].Journal of Earth Sciences and Environment,2018,40(4):473-486.
[3] FORNASARO S,MORELLI G,RIMONDI V,et al.Mercury Distribution Around the Siele Hg Mine(Mt.Amiata District,Italy)Twenty Years After Reclamation:Spatial and Temporal Variability in Soil,Stream Sediments,and Air[J].Journal of Geochemical Exploration,2022,232:375-6742.
[4] 卢光华,岳昌盛,彭 犇,等.汞污染土壤修复技术的研究进展[J].工程科学学报,2017,39(1):1-12.
LU Guang-hua,YUE Chang-sheng,PENG Ben,et al.Review of Research Progress on the Remediation Te-chnology of Mercury Contaminated Soil[J].Chinese Journal of Engineering,2017,39(1):1-12.
[5] 魏 赢,刘阳生.汞污染农田土壤的化学稳定化修复[J].环境工程学报,2017,11(3):1878-1884.
WEI Ying,LIU Yang-sheng.Remediation on Mercury Polluted Farmland Soil by Chemical Stabilization[J].Chinese Journal of Environmental Engineering,2017,11(3):1878-1884.
[6] 张召阳.我国表层土壤中汞和硒的分布特征及形成机制研究[D].北京:中国科学院大学,2021.
ZHANG Zhao-yang.Distribution Characteristics and Formation Mechanism of Mercury and Selenium in Topsoil of China[D].Beijing:University of Chinese Academy of Sciences,2021.
[7] 成杭新,庄广民,赵传冬,等.北京市土壤Hg污染的区域生态地球化学评价[J].地学前缘,2008,15(5):126-145.
CHENG Hang-xin,ZHUANG Guang-min,ZHAO Chuan-dong,et al.Regional Eco-geochemical Assessment of Mercury in Soils in Beijing[J].Earth Science Frontiers,2008,15(5):126-145.
[8] 高令健,毛 康,张 伟,等.贵州万山汞矿区稻田土壤汞的分布及污染特征[J].矿物岩石地球化学通报,2021,40(1):148-154.
GAO Ling-jian,MAO Kang,ZHANG Wei,et al.Temporal and Spatial Distribution and Pollution Characteristics of Mercury in Paddy Soils of the Wanshan Mercury Mining Area,Guizhou Province[J].Bulletin of Mineralogy,Petrology and Geochemistry,2021,40(1):148-154.
[9] 张 琦,郭庆军,陶正华.长江流域汞的生物地球化学研究进展[J].生态学杂志,2021,40(6):1861-1873.
ZHANG Qi,GUO Qing-jun,TAO Zheng-hua.Advances in Biogeochemistry of Mercury in the Yangtze River Basin[J].Chinese Journal of Ecology,2021,40(6):1861-1873.
[10] ACQUAVITA A,BRANDOLIN D,CATTARUZZA C,et al.Mercury Distribution and Speciation in Historically Contaminated Soils of the Isonzo River Plain(NE Italy)[J].Journal of Soils and Sediments,2022,22(1):79-92.
[11] 黄 勇,段续川,袁国礼,等.北京市延庆区土壤重金属元素地球化学特征及其来源分析[J].现代地质,2022,36(2):634-644.
HUANG Yong,DUAN Xu-chuan,YUAN Guo-li,et al.Geochemistry and Source Identification of Heavy Me-tals in the Top and Subsoil of Yanqing District in Beijing[J].Geoscience,2022,36(2):634-644.
[12] 李 苹,黄 勇,林 赟,等.北京市怀柔区土壤重金属的分布特征、来源分析及风险评价[J].现代地质,2018,32(1):86-94.
LI Ping,HUANG Yong,LIN Yun,et al.Distribution,Source Identification and Risk Assessment of Heavy Metals in Topsoil of Huairou District in Beijing[J].Geoscience,2018,32(1):86-94.
[13] 张沁瑞,李 欢,邓宇飞,等.北京东南郊土壤重金属元素分布及其在表层土壤中的富集特征[J].物探与化探,2022,46(2):490-501.
ZHANG Qin-rui,LI Huan,DENG Yu-fei,et al.Distribution of Heavy Metal Elements in Soil of the Southeastern Suburbs of Beijing and Their Enrichment Characteristics in Surface Soil[J].Geophysical and Geochemical Exploration,2022,46(2):490-501.
[14] 索琳娜,刘宝存,赵同科,等.北京市菜地土壤重金属现状分析与评价[J].农业工程学报,2016,32(9):179-186.
SUO Lin-na,LIU Bao-cun,ZHAO Tong-ke,et al.Evaluation and Analysis of Heavy Metals in Vegetable Field of Beijing[J].Transactions of the Chinese Society of Agricultural Engineering,2016,32(9):179-186.
[15] 杨少斌,于 鑫,孙向阳,等.北京城区绿地土壤重金属污染评价与空间分析[J].生态环境学报,2018,27(5):933-941.
YANG Shao-bin,YU Xin,SUN Xiang-yang,et al.Pollution Assessment and Spatial Structure Analysis of Heavy Metals of Greenbelt Soil in Beijing Urban Area[J].Ecology and Environmental Sciences,2018,27(5):933-941.
[16] 李 欢,黄 勇,张沁瑞,等.北京平原区土壤地球化学特征及影响因素分析[J].物探与化探,2021,45(2):502-516.
LI Huan,HUANG Yong,ZHANG Qin-rui,et al.Soil Geochemical Characteristics and Influencing Factors in Beijing Plain[J].Geophysical and Geochemical Exploration,2021,45(2):502-516.
[17] 黄 勇,杨忠芳,冯 辉,等.北京城区24年来土壤Hg元素时空变异特征[J].现代地质,2014,28(5):935-941.
HUANG Yong,YANG Zhong-fang,FENG Hui,et al.Characteristics of Spatio-temporal Variability of Soil Mercury in Beijing Urban for 24 Years[J].Geoscience,2014,28(5):935-941.
[18] 党 莹,张小玲,饶晓琴,等.北京与成都大气污染特征及空气质量改善效果评估[J].环境科学,2021,42(8):3622-3632.
DANG Ying,ZHANG Xiao-ling,RAO Xiao-qin,et al.Evaluation of Air Pollution Characteristics and Air Quality Improvement Effect in Beijing and Chengdu[J].Environmental Science,2021,42(8):3622-3632.
[19] 杨文杰,赵信如,巩前文.北京“百万亩造林”对浅山区生物多样性的影响评价[J].中国农业资源与区划,2020,41(4):83-93.
YANG Wen-jie,ZHAO Xin-ru,GONG Qian-wen.Biodiversity Impact Assessment of “One Million Mu Afforestation” in the Shallow Mountain Area of Beijing[J].Chinese Journal of Agricultural Resources and Regional Planning,2020,41(4):83-93.
[20] DZ/T 0258—2014,多目标区域地球化学调查规范(1:250 000)[S].
DZ/T 0258—2014,Specification of Multi-purpose Regional Geochemical Survey(1:250 000)[S].
[21] DD2005-03,生态地球化学评价样品分析技术要求[S].
DD2005-03,Technical Requirements for Analysis of Ecological Geochemical Evalution Samples[S].
[22] 成杭新,李 括,李 敏,等.中国城市土壤化学元素的背景值与基准值[J].地学前缘,2014,21(3):265-306.
CHENG Hang-xin,LI Kuo,LI Min,et al.Geochemical Background and Baseline Value of Chemical Elements in Urban Soil in China[J].Earth Science Frontiers,2014,21(3):265-306.
[23] 黎恒明,杨苗苗.汉江中游典型小流域土壤有效锌空间变异特征及评价[J].地球科学与环境学报,2016,38(5):700-707.
LI Heng-ming,YANG Miao-miao.Spatial Variation Characteristics and Evaluation of Soil Available Zinc in a Typical Small Watershed of the Middle Hanjiang River[J].Journal of Earth Sciences and Environment,2016,38(5):700-707.
[24] 倪碧珩,陆 胤,施维林.土壤重金属元素含量的预测方法仿真研究[J].计算机仿真,2022,39(5):234-237.
NI Bi-heng,LU Yin,SHI Wei-lin.Simulation Study on Prediction Method of Soil Heavy Metal Content[J].Computer Simulation,2022,39(5):234-237.
[25] 张皓月,刘文波,张绪教,等.河套平原地下水中砷的空间变异特征及影响因素分析[J].地质科技通报,2021,40(1):192-199.
ZHANG Hao-yue,LIU Wen-bo,ZHANG Xu-jiao,et al.Analysis of Spatial Variability and Influencing Factors of Arsenic in Groundwater of Hetao Plain,Inner Mongolia[J].Bulletin of Geological Science and Technology,2021,40(1):192-199.
[26] 侯青叶,杨忠芳,余 涛,等.中国土壤地球化学参数[M].北京:地质出版社,2020.
HOU Qing-ye,YANG Zhong-fang,YU Tao,et al.Soil Geochemical Parameters in China[M].Beijing:Geological Publishing House,2020.
[27] 杨忠芳,侯青叶,余 涛,等.农田生态系统区域生态地球化学评价的示范研究:以成都经济区土壤Cd为例[J].地学前缘,2008,15(5):23-35.
YANG Zhong-fang,HOU Qing-ye,YU Tao,et al.An Example of Eco-geochemical Assessment for Agroe-cosystems:A Study of Cd in Chengdu Economic Region[J].Earth Science Frontiers,2008,15(5):23-35.
[28] WANG Z J,WANG L,ZHANG G,et al.Characteristics of Mercury Pollution and Ecological Risk Assessment in Different Degraded Grasslands of the Songnen Plains,Northeastern China[J].Sustainability,2021,13(19):1050-2071.
[29] 北京市统计局.北京统计年鉴2020[M].北京:中国统计出版社,2020.
Beijing Municipal Bureau Statistics.Beijing Statistical Yearbook 2020[M].Beijing:China Statistics Press,2020.
[30] 北京市生态环境局.北京市2017年环境统计年报[R].北京:北京市生态环境局,2017.
Beijing Municipal Ecology and Environment Bureau.Beijing Municipal Environmental Statistics Annual Report 2017[R].Beijing:Beijing Municipal Ecology and Environment Bureau,2017.
[31] 李 珊,李 洋,梁汉东,等.北京城郊燃煤汞排放及其对当地空气环境的影响[J].环境科学研究,2014,27(12):1420-1425.
LI Shan,LI Yang,LIANG Han-dong,et al.Atmospheric Mercury Emissions from Domestic Coal and Impacts on Local Environment of Suburban Beijing[J].Research of Environmental Sciences,2014,27(12):1420-1425.
[32] 丛 源,陈岳龙,杨忠芳,等.北京平原区元素的大气干湿沉降通量[J].地质通报,2008,27(2):257-264.
CONG Yuan,CHEN Yue-long,YANG Zhong-fang,et al.Dry and Wet Atmospheric Deposition Fluxes of Elements in the Plain Area of Beijing Municipality,China[J].Geological Bulletin of China,2008,27(2):257-264.
[33] 黄 勇,李 欢,孙 朝,等.北京市土壤地质环境监测网建设成果报告[R].北京:北京市生态地质研究所,2018.
HUANG Yong,LI Huan,SUN Zhao,et al.Report on the Construction of Soil Geological Environment Monitoring Network in Beijing[R].Beijing:Beijing Institute of Ecological Geology,2018.
[34] 曾晓舵,王向琴,凃新红,等.农田土壤重金属污染阻控技术研究进展[J].生态环境学报,2019,28(9):1900-1906.
ZENG Xiao-duo,WANG Xiang-qin,TU Xin-hong,et al.Research Progress on Speciation and Physiological Control of Heavy Metal in Soil-plant System[J].Eco-logy and Environmental Sciences,2019,28(9):1900-1906.
[35] 谭清友,付学吾,何天容.我国自然源汞排放研究进展[J].生态学杂志,2017,36(3):833-845.
TAN Qing-you,FU Xue-wu,HE Tian-rong.Mercury Emission from Natural Sources in China:A Critical Review[J].Chinese Journal of Ecology,2017,36(3):833-845.
[36] 李天魁,刘 毅,王超然,等.基于离散选择模型的北京市工业疏解环境影响[J].清华大学学报(自然科学版),2017,57(11):1163-1169.
LI Tian-kui,LIU Yi,WANG Chao-ran,et al.Environmental Impact of Beijing's Industrial Decentralization Based on a Discrete Choice Modeling Approach[J].Journal of Tsinghua University(Science and Techno-logy),2017,57(11):1163-1169.
[37] 韩 鹏.北京市首钢地区土壤重金属分布及土壤质量评价[D].北京:中国地质大学,2012.
HAN Peng.The Distribution of Heavy Metals and Assessment of Soil Quality in Capital Steel Factory in Beijing,China[D].Beijing:China University of Geosciences,2012.
[38] 孙天河.北京东南郊化工区土壤中重金属元素的环境地球化学研究[D].北京:中国地质大学,2013.
SUN Tian-he.The Study of Heavy Metals in the Soil of South-eastern Suburb Chemical Industry Zone in Beijing[D].Beijing:China University of Geosciences,2013.
[39] 安永龙,黄 勇,刘清俊,等.北京城区表层土壤多元素分布特征及重金属元素污染评价[J].地质通报,2016,35(12):2111-2120.
AN Yong-long,HUANG Yong,LIU Qing-jun,et al.The Distribution of Surface Soil Elements and the Pollution Assessment of Heavy Metal Elements in Beijing[J].Geological Bulletin of China,2016,35(12):2111-2120.
[40] 王京文,谢国雄,章明奎.大气沉降对萝卜地上和地下部分铅镉汞砷积累的影响[J].土壤通报,2018,49(1):184-190.
WANG Jing-wen,XIE Guo-xiong,ZHANG Ming-kui.Effects of Atmospheric Deposition on the Accumulation of Lead,Cadmium,Mercury and Arsenic in Abo-veground and Underground Parts of Radish[J].Chinese Journal of Soil Science,2018,49(1):184-190.
[41] 于向楠,李飞扬,符耿雪,等.北京市道路尘中重金属时空分布特征及污染程度评价[J].现代地质,2019,33(1):169-175.
YU Xiang-nan,LI Fei-yang,FU Geng-xue,et al.The Spatial-temporal Distribution Characteristics and Contamination Assessments of Heavy Metals in the Road Dusts of Beijing[J].Geoscience,2019,33(1):169-175.
[42] 刘俊华,王文华,彭 安.北京市二个主要工业区汞污染及其来源的初步研究[J].环境科学学报,1998,18(3):109-114.
LIU Jun-hua,WANG Wen-hua,PENG An.Pollution and Sources of Hg in Top Soil in Two District of Beijing City[J].Acta Scientiae Circumstantiae,1998,18(3):109-114.
[43] 熊定国,廖 激.四川省环境中的汞[J].四川环境,1994,13(1):46-49.
XIONG Ding-guo,LIAO Ji.Mercury in the Environment of Sichuan Province[J].Sichuan Environment,1994,13(1):46-49.

相似文献/References:

[1]奥 勇,毋冰龙,白召弟,等.基于类NPP-VIIRS夜间灯光数据的粤港澳大湾区城市建成区时空动态特征[J].地球科学与环境学报,2022,44(03):513.[doi:10.19814/j.jese.2021.12040]
 AO Yong,WU Bing-long,BAI Zhao-di,et al.Temporal-spatial Changes of Urban Built-up Area Expansion in Guangdong-Hong Kong-Macao Greater Bay Area, China Based on NPP-VIIRS-like Night Light Data[J].Journal of Earth Sciences and Environment,2022,44(01):513.[doi:10.19814/j.jese.2021.12040]
[2]杜国明,孙嘉曼,李玉恒*.东北黑土地产能时空演变及其提升对策[J].地球科学与环境学报,2023,45(02):338.[doi:10.19814/j.jese.2022.04044]
 DU Guo-ming,SUN Jia-man,LI Yu-heng*.Spatio-temporal Evolution of Black Cropland Productivity in Northeast China and Its Promotion Countermeasures[J].Journal of Earth Sciences and Environment,2023,45(01):338.[doi:10.19814/j.jese.2022.04044]

备注/Memo

备注/Memo:
收稿日期:2022-10-23; 修回日期:2022-12-18投稿网址:http:∥jese.chd.edu.cn/
基金项目:北京市地质勘探基金项目(11000022T000000439575,11000022T000000491145)
作者简介:李 欢(1990-),男,黑龙江绥化人,工程师,E-mail:lihuan_8@163.com。
*通讯作者:张沁瑞(1980-),男,山西长治人,高级工程师,E-mail:18601040279@163.com。
更新日期/Last Update: 2023-01-30