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《地球科学与环境学报》[ISSN:1672-6561/CN:61-1423/P]

卷:

第33卷

期数:

2011年第02期

页码:

177-184

栏目:

资源与环境

出版日期:

2011-06-15

文章信息/Info

Title:

Research Significance and Role of Black Carbon in the Global Climate and Environmental Systems

文章编号:

1672-6561(2011)02-0177-08

作者:

曹军骥¹; 2; 占长林¹; 3

1.中国科学院地球环境研究所 黄土与第四纪地质国家重点实验室,陕西 西安 710075; 2.西安交通大学 全球环境变化研究院,陕西 西安 710049; 3.西安交通大学 机械工程学院,陕西 西安 710049

Author(s):

CAO Jun-ji¹; 2; ZHAN Chang-lin¹; 3

1. State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences,Xi'an 710075, Shaanxi, China; 2. Institute of Global Environmental Change, Xi'an Jiaotong University, Xi'an 710049,Shaanxi, China; 3. Scho

关键词:

黑碳; 降解; 全球碳循环; 有机碳; 土壤; 沉积物; 气候变化; 火事件

Keywords:

black carbon;  degradation;  global carbon cycle;  organic carbon;  soil;  sediments;  climate change;  fire regime

分类号:

P532

DOI:

-

文献标志码:

A

摘要:

燃烧形成的黑碳粒子进入大气中可影响辐射平衡,导致全球气候变暖,其沉降在河流、湖泊、海洋、土壤等环境中对全球生物地球化学循环起到重要的作用,成为当前国际地球科学研究的热点问题。综述了黑碳的定义及排放、沉降、降解过程,并总结了其在现在及过去环境和气候系统中的重要作用与研究意义。黑碳是全球惰性有机碳库的重要组成部分,在全球慢速碳循环中发挥潜在作用。因其具有很强的吸光特性,它在区域气候变暖过程中扮演重要角色。沉降在不同地质载体中的黑碳难以降解,可以保存几百万年,为地质历史时期古气候和古环境重建研究提供重要信息。海洋沉积物过去数百万年的黑碳记录指示了天然火的演化信息,晚第四纪黄土剖面黑碳也指示了天然火的变化信息,最近千年的湖泊和冰芯黑碳记录既反映了天然火的信息,也指示人类活动的信号。未来黑碳研究应进一步关注标准测量方法,以真正理解黑碳在全球气候与环境系统中的作用。

Abstract:

Black carbon(BC)particles emit into the atmosphere during the combustion process, which can directly affect the radiation balance, leading to global warming. BC that deposited in the rivers, lakes, oceans and soils plays an important role in the global biogeochemical cycles. It became a hot topic in the international geoscience research. The definition, emissions, deposition and degradation processes of BC were reviewed, and its important role and research significance in the present and past environment and climate system were summarized. BC is an important component of the inert carbon pool and it was involved in the global slow carbon cycle. Due to its strong adsorption properties, BC exerts positive impact on the regional climate warming. Since it is difficult to degrade, BC can be stored for millions of years, which provides clue for the reconstructions of paleoclimate and paleoenvironment. BC records from marine sediments indicated the evolution of natural fire over the past few million years. BC records from the Late Quaternary loess sections also showed the variation of natural fire. BC records from lacustrines and ice cores over the recent thousand years not only reflected the changes of natural fire, but also implied the signals of human activities. Future research should pay more attentions to standard measurement methods, and then the function of black carbon could be truly understood in the global climate and environment systems.

参考文献/References:

[1] IPCC.Intergovernmental Panel on Climate Change,Climate Change[M].Cambridge:Cambridge University Press,2007.
[2] Jacobson M Z.Strong Radiative Heating Due to the Mixing State of Black Carbon in Atmospheric Aerosols[J].Nature,2001,409:695-697.
[3] Menon S,Hansen J,Nazarenko L,et al.Climate Effects of Black Carbon Aerosols in China and India[J].Science,2002,297:2250-2253.
[4] Venkataraman C,Habib G,Eiguren-Fernandez A,et al.Residential Biofuels in South Asia:Carbonaceous Aerosol Emissions and Climate Impacts[J].Science,2005,307:1454-1456.
[5] Gustafsson Ö,Krusa M,Zencak Z,et al.Brown Clouds over South Asia:Biomass or Fossil Fuel Combustion?[J].Science,2009,323:495-498.
[6] Wolbach W S,Gilmour I,Anders E,et al.Global Fire at the Cretaceous:Tertiary Boundary[J].Nature,1988,334:665-669.
[7] Cope M J,Chaloner W G.Fossil Charcoal as Evidence of Past Atmospheric Composition[J].Nature,1980,283:647-649.
[8] Belcher C M,McElwain J C.Limits for Combustion in Low O₂ Redefine Paleoatmospheric Predictions for the Mesozoic[J].Science,2008,321:1197-1200.
[9] Kuhlbusch T A J.Ocean Chemistry:Black Carbon and the Carbon Cycle[J].Science,1998,280:1903-1904.
[10] Masiello C A,Druffel E R.Black Carbon in Deep-sea Sedi-ments[J].Science,1998,280:1911-1913.
[11] Masiello C A.New Directions in Black Carbon Organic Geochemistry[J].Marine Chemistry,2004,92(1/2):201-213.
[12] Hammes K,Schmidt M W I,Smernik R J,et al.Comparison of Quantification Methods to Measure Fire-derived(Black/elemental)Carbon in Soils and Sediments Using Reference Materials from Soil,Water,Sediment and the Atmosphere[J].Global Biogeochemical Cycles,2007,21(GB3016).DOI:10.1029/2006GB002914.
[13] Lynch A H,Beringer J,Kershaw P,et al.Using the Paleorecord to Evaluate Climate and Fire Interactions in Australia[J].Annual Review of Earth and Planetary Sciences,2007,35:215-239.
[14] DeLuca T H,Aplet G H.Charcoal and Carbon Storage in Forest Soils of the Rocky Mountain West[J].Frontiers in Ecology and the Environment,2008,6(1):18-24.
[15] Goldberg E.Black Carbon in the Environment[M].New York:John Wiley and Sons,1985.
[16] Hedges J I,Eglinton G,Hatcher P G,et al.The Molecularly-uncharacterized Component of Nonliving Organic Matter in Natural Environments[J].Organic Geochemistry,2000,31(10):945-958.
[17] Liang B Q,Lehmann J,Solomon D,et al.Stability of Biomass-derived Black Carbon in Soils[J].Geochimica et Cosmochimica Acta,2008,72(24):6069-6078.
[18] Streets D G,Gupta S,Waldhoff S T,et al.Black Carbon Emissions in China[J].Atmospheric Environment,2001,35(25):4281-4296.
[19] Chameides W L,Bergin M.Climate Change:Soot Takes Center Stage[J].Science,2002,297:2214-2215.
[20] Gelencsér A.Carbonaceous Aerosol[M].New York:Springer-Verlag,2005.
[21] Schmidt M W.Biogeochemistry:Carbon Budget in the Black[J].Nature,2004,427:305-307.
[22] Czimczik C I,Schmidt M W I,Schulze E D.Effects of Increasing Fire Frequency on Black Carbon and Organic Matter in Podzols of Siberian Scots Pine Forests[J].European Journal of Soil Science,2005,56(3):417-428.
[23] Middelburg J J,Nieuwenhuize J,VanBreugel P.Black Carbon in Marine Sediments[J].Marine Chemistry,1999,65(3/4):245-252.
[24] Bird M I,Moyo C,Veenendaal E M,et al.Stability of Elemental Carbon in a Savanna Soil[J].Global Biogeochemical Cycles,1999,13(4):923-932.
[25] Mannino A,Harvey H R.Black Carbon in Estuarine and Coastal Ocean Dissolved Organic Matter[J].Limnology and Oceanography,2004,49(3):735-740.
[26] Baldock J A,Smernik R J.Chemical Composition and Bio-availability of Thermally Altered Pinus Resinosa(Red Pine)Wood[J].Organic Geochemistry,2002,33(9):1093-1109.
[27] Seiler W,Crutzen P J.Estimates of Gross and Net Fluxes of Carbon Between the Biosphere and the Atmosphere from Biomass Burning[J].Climatic Change,1980,2(3):207-247.
[28] Crutzen P J,Andreae M O.Biomass Burning in the Tropics:Impact on Atmospheric Chemistry and Biogeochemical Cycles[J].Science,1990,250:1669-1678.
[29] Kuhlbusch T A J,Crutzen P J.Toward a Global Estimate of Black Carbon in Residues of Vegetation Fires Representing a Sink of Atmospheric CO₂ and a Source of O₂[J].Global Biogeochemical Cycles,1995,9(4):491-501.
[30] Preston C M.Biogeochemistry:Fire's Black Legacy[J].Nature Geoscience,2009,2(10):674-675.
[31] Druffel E R M.Comments on the Importance of Black Carbon in the Global Carbon Cycle[J].Marine Chemistry,2004,92(1/2):197-200.
[32] Dickens A F,Gélinas Y,Masiello C A,et al.Reburial of Fossil Organic Carbon in Marine Sediments[J].Nature,2004,427:336-339.
[33] 韩永明,曹军骥.环境中的黑碳及其全球生物地球化学循环[J].海洋地质与第四纪地质,2005,25(1):125-132.
[34] Hockaday W C.The Organic Geochemistry of Charcoal Black Carbon in the Soils of the University of Michigan Biological Station[D].Columbus:The Ohio State University,2006.
[35] Ackerman A S,Toon O B,Stevens D E,et al.Reduction of Tropical Cloudiness by Soot[J].Science,2000,288:1042-1047.
[36] Ramanathan V,Carmichael G.Global and Regional Climate Changes Due to Black Carbon[J].Nature Geoscience,2008,1(4):221-227.
[37] Wang C.A Modeling Study on the Climate Impacts of Black Carbon Aerosols[J].Journal of Geophysical Research,2004,109(D03106).DOI:10.1029/2003JD004084.
[38] Jacobson M Z.Control of Fossil-fuel Particulate Black Carbon and Organic Matter,Possibly the Most Effective Method of Slowing Global Warming[J].Journal of Geophysical Research,2002,107(4410).DOI:10.1029/2001JD001376.
[39] Sander M,Pignatello J J.Characterization of Charcoal Ad-sorption Sites for Aromatic Compounds:Insights Drawn from Single-solute and Bi-solute Competitive Experiments[J].Environment Science Technology,2005,39(6):1606-1615.
[40] Czimczik C I,Preston C M,Schmidt M W I,et al.How Surface Fire in Siberian Scots Pine Forests Affects Soil Organic Carbon in the Forest Floor:Stocks,Molecular Structure,and Conversion to Black Carbon[J].Global Biogeochemical Cycles,2003,17.DOI:10.1029/2002GB001956.
[41] Piccolo A,Spaccini R,Nieder R,et al.Sequestration of a Biologically Labile Organic Carbon in Soils by Humified Organic Matter[J].Climatic Change,2004,67(2/3):329-343.
[42] Marris E.Putting the Carbon Back:Black Is the New Green[J].Nature,2006,442:624-626.
[43] Smith D M,Griffin J J,Goldberg E D.Elemental Carbon in Marine Sediments:a Baseline for Burning[J].Science,1973,241:268-270.
[44] Verardo D J,Ruddiman W F.Late Pleistocene Charcoal in Tropical Atlantic Deep-sea Sediments:Climatic and Geochemi-cal Significance[J].Geology,1996,24(9):855-857.
[45] Bird M I,Cali J A.A Million-year Record of Fire in Sub-Saharan Africa[J].Nature,1998,394:767-769.
[46] Jia G D,Peng P A,Zhao Q H,et al.Changes in Terrestrial Ecosystem Since 30 Ma in East Asia:Stable Isotope Evidence from Black Carbon in the South China Sea[J].Geology,2003,31(12):1093-1096.
[47] 刘东生.黄土与环境[M].北京:科学出版社,1985.
[48] An Z S.The History and Variability of the East Asian Paleomonsoon Climate[J].Quaternary Science Reviews,2000,19(1/2):171-187.
[49] An Z S,Kutzbach J E,Prell W L,et al.Evolution of Asian Monsoons and Phased Uplift of the Himalaya-Tibetan Plateau Since Late Miocene Times[J].Nature,2001,411:62-66.
[50] Yang Y,Shen C D,Yi W X,et al.The Elemental Carbon Record in Weinan Loess Section Since the Last 21 ka[J].Chinese Science Bulletin,2001,46(18):1541-1543.
[51] Wang X,Peng P A,Ding Z L.Black Carbon Records in Chinese Loess Plateau over the Last Two Glacial Cycles and Implications for Paleofires[J].Palaeogeography,Palaeoclimatology,Palaeoecology,2005,223(1/2):9-19.
[52] Zhou B,Shen C D,Sun W D,et al.Elemental Carbon Record of Paleofire History on the Chinese Loess Plateau During the Last 420 ka and Its Response to Environmental and Climate Changes[J].Palaeogeography,Palaeoclimatology,Palaeoecology,2007,252(3/4):617-625.
[53] Long C J,Whitlock C,Bartlein P J,et al.A 9000-year Fire History from the Oregon Coast Range,Based on a High-resolution Charcoal Study[J].Canadian Journal of Forest Research,1998,28(5):774-787.
[54] Muri G,Cermelj B,Faganeli J,et al.Black Carbon in Slovenian Alpine Lacustrine Sediments[J].Chemosphere,2002,46(8):1225-1234.
[55] 韩永明,曹军骥,金章东,等.岱海与太湖沉积物焦碳和烟炱最近200年历史对比研究[J].第四纪研究,2010,30(3):550-558.
[56] Clarke A D,Noone K J.Soot in the Arctic Snowpack:a Cause for Perturbations in Radiative Transfer[J].Atmospheric Environment,1985,19(12):2045-2053.
[57] Cachier H,Pertuisot M H.Particulate Carbon in Arctic Ice:Ice Archives in Antarctica and Greenland[J].Analusis,1994,22(7):34-37.
[58] Chylek P,Johnson B,Damiano P A,et al.Biomass Burning Record and Black Carbon in the GISP2 Ice Core[J].Geophysical Research Letters,1995,22(2):89-92.
[59] Lavanchy V M H,Gäggeler H W,Schotterer U,et al.Historical Record of Carbonaceous Particle Concentrations from a European High-alpine Glacier(Colle Gnifetti,Switzerland)[J].Journal of Geophysical Research,1999,104(D17):21227-21236.
[60] McConnell J R,Edwards R,Kok G L,et al.20th-century Industrial Black Carbon Emissions Altered Arctic Climate Forcing[J].Science,2007,317:1381-1384.
[61] Ming J,Cachier H,Xiao C,et al.Black Carbon Record Based on a Shallow Himalayan Ice Core and Its Climatic Implications[J].Atmospheric Chemistry and Physics,2008,8(5):1343-1352.
[62] Xu B Q,Cao J J,Hansen J,et al.Black Soot and the Survival of Tibetan Glaciers[J].Proceedings of the National Academy of Sciences,2009,106(52):22114-22118.

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备注/Memo

备注/Memo:

收稿日期:2011-01-04
基金项目: 国家自然科学杰出青年基金项目(40925009)
作者简介: 曹军骥(1971-),男,湖北鄂州人,研究员,博士研究生导师,理学博士,从事第四纪地质学和大气化学研究。E-mail:cao@loess.llqg.ac.cn

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更新日期/Last Update: 2011-06-20