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Characteristics of Aerosol Pollution and Particle Size Distribution Evolution During a Dust Storm Process in 2024 in Xi’an Area of Shaanxi, China(PDF)

《地球科学与环境学报》[ISSN:1672-6561/CN:61-1423/P]

Issue:
2025年第04期
Page:
844-856
Research Field:
黄河流域生态保护和高质量发展专刊(下)
Publishing date:

Info

Title:
Characteristics of Aerosol Pollution and Particle Size Distribution Evolution During a Dust Storm Process in 2024 in Xi’an Area of Shaanxi, China
Author(s):
ZHONG Jia-haoWANG Si-yuWANG YanZHANG Li-yuan*
(School of Water and Environment, Chang’an University, Xi’an 710064, Shaanxi, China)
Keywords:
dust storm atmospheric particulate matter pollutant particle size distribution inorganic component analysis PMF source apportionment aerosol Shaanxi
PACS:
X513
DOI:
10.19814/j.jese.2025.02035
Abstract:
To investigate the characteristics of aerosol pollution and particle size distribution evolution during a dust storm process in Xi’an area of Shaanxi from March 15th to 17th, 2024, an optical particle sizer and an online environmental ion monitor were employed to observe the dynamic changes in particle size distribution and ion composition of atmosphere; combined with atmospheric pollutant data and meteorological data, the characteristics of particulate matter pollution and particle size distribution evolution during the dust storm process were studied. The results show that the dust storm process is divided into four periods, including clean background period, the first period of the dust storm process(dust period Ⅰ), the secondary period of the dust storm process(dust period Ⅱ), and dust dissipation period; significant differences are observed in aerosol sources, particle size distribution, and ion composition across these periods; compared with the clean background period, the particle mass concentration do not show a significant increase during dust period Ⅰ, but the particle number concentration with sizes 0.300 μm to 0.576 μm ranging from increases rapidly; the ionic composition is dominated by NH+4 and secondary pollutants such as NO-3 and SO2-4; in dust period Ⅱ, the coarse particles with sizes larger than 2.5 μm become dominant; the particle number concentration decreases, while the mass concentrations of Ca2+, Mg2+, and Na+ increase several times; compared with clean background period, dust period Ⅰ is dominated by smaller particles, causing the particle size spectrum to shift upward; compared with dust period Ⅰ, dust period Ⅱ is dominated by larger particles, resulting in a rightward shift of peak particle size. Backward trajectory analysis and PMF source apportionment results indicate that particle pollution during dust period Ⅰ is mainly attributed to anthropogenic pollution sources from satellite towns and suburbs around Xi’an city, while dust period Ⅱ exhibits clear characteristics of dust sources.

References:

[1] 张仁健,韩志伟,王明星,等.中国沙尘暴天气的新特征及成因分析[J].第四纪研究,2002,22(4):374-380.
ZHANG Ren-jian,HAN Zhi-wei,WANG Ming-xing,et al.Dust Storm Weather in China:New Characteristics and Origins[J].Quaternary Sciences,2002,22(4):374-380.
[2] ZHANG C,YAN M L,DU H,et al.Mortality Risks from a Spectrum of Causes Associated with Sand and Dust Storms in China[J].Nature Communications,2023,14(1):6867.
[3] 叶燕华,张 宁,王基鑫,等.兰州市一次持续重污染过程的气象条件分析[J].中国环境科学,2023,43(12):6281-6289.
YE Yan-hua,ZHANG Ning,WANG Ji-xin,et al.Analysis of Meteorological Conditions of a Continuous Heavy Pollution Process Affecting Lanzhou[J].China Environmental Science,2023,43(12):6281-6289.
[4] 张 喆,丁建丽,王瑾杰.中亚沙尘气溶胶时空分布特征及潜在扩散特性分析[J].地理学报,2017,72(3):507-520.
ZHANG Zhe,DING Jian-li,WANG Jin-jie.Spatio-temporal Variations and Potential Diffusion Characteristics of Dust Aerosol Originating from Central Asia[J].Acta Geographica Sinica,2017,72(3):507-520.
[5] 申莉莉,盛立芳,陈静静.一次强沙尘暴过程中沙尘气溶胶空间分布的初步分析[J].中国沙漠,2010,30(6):1483-1490.
SHEN Li-li,SHENG Li-fang,CHEN Jing-jing.Preliminary Analysis of the Spatial Distribution of the Dust Aerosol in a Heavy Dust Storm[J].Journal of Desert Research,2010,30(6):1483-1490.
[6] HILL W,LIM E L,WEEDEN C E,et al.Lung Adenocarcinoma Promotion by Air Polltants[J].Nature,2023,616:159-167.
[7] 赵留元,李子璇,吕沛诚,等.基于SPAMS的兰州市2018年冬季沙尘天气过程细颗粒物污染特征及来源研究[J].环境科学学报,2020,40(2):388-400.
ZHAO Liu-yuan,LI Zi-xuan,LYU Pei-cheng,et al.Pollution Characteristics and Sources of Atmospheric Fine Particulates During the Period of 2018,Winter Dust Weather in Lanzhou City Based on SPAMS Te-chnology[J].Acta Scientiae Circumstantiae,2020,40(2):388-400.
[8] NI R J,SU H,BURNETT R T,et al.Long-term Exposure to PM2.5 Has Significant Adverse Effects on Childhood and Adult Asthma:A Global Meta-analysis and Health Impact Assessment[J].One Earth,2024,7(11):1953-1969.
[9] YIN Z C,WAN Y,ZHANG Y J,et al.Why Super Sandstorm 2021 in North China?[J].National Scien-ce Review,2022,9(3):nwab165.
[10] ZUO P J,HUANG Y M,LIU P F,et al.Stable Iron Isotopic Signature Reveals Multiple Sources of Magnetic Particulate Matter in the 2021 Beijing Sandstorms[J].Environmental Science & Technology Letters,2022,9(4):299-305.
[11] DILLNER A M,SCHAUER J J,ZHANG Y H,et al.Size-resolved Particulate Matter Composition in Beijing During Pollution and Dust Events[J].Journal of Geophysical Research:Atmospheres,2006,111(D5):2005JD006400.
[12] ZHOU C H,GUI H L,HU J K,et al.Detection of New Dust Sources in Central/East Asia and Their Im-pact on Simulations of a Severe Sand and Dust Storm[J].Journal of Geophysical Research:Atmospheres,2019,124(17/18):10232-10247.
[13] KRASNOV H,KATRA I,FRIGER M.Increase in Dust Storm Related PM10 Concentrations:A Time Series Analysis of 2001-2015[J].Environmental Pollution,2016,213:36-42.
[14] PROSPERO J M.Long-range Transport of Mineral Dust in the Global Atmosphere:Impact of African Dust on the Environment of the Southeastern United States[J].PNAS,1999,96(7):3396-3403.
[15] TANG K,HUANG Z W,HUANG J P,et al.Characterization of Atmospheric Bioaerosols Along the Tran-sport Pathway of Asian Dust During the Dust-bioaerosol 2016 Campaign[J].Atmospheric Chemistry and Physics,2018,18(10):7131-7148.
[16] YU G Y,QIN X F,XU J,et al.Characteristics of Particulate-bound Mercury at Typical Sites Situated on Dust Transport Paths in China[J].Science of the Total Environment,2019,648:1151-1160.
[17] WANG Y,ZHUANG G S,TANG A H,et al.The Evolution of Chemical Components of Aerosols at Fi-ve Monitoring Sites of China During Dust Storms[J].Atmospheric Environment,2007,41(5):1091-1106.
[18] ZHANG X L,ZHAO L J,TONG D Q,et al.A Systematic Review of Global Desert Dust and Associated Human Health Effects[J].Atmosphere,2016,7(12):158.
[19] 霍 文,何 清,杨兴华,等.中国北方主要沙漠沙尘粒度特征比较研究[J].水土保持研究,2011,18(6):6-11.
HUO Wen,HE Qing,YANG Xing-hua,et al.The Re-search on Grain Size Characteristic of Desert in North of China[J].Research of Soil and Water Conservation,2011,18(6):6-11.
[20] 张延伟,唐湘玲,陆 辉,等.2012年春季塔克拉玛干沙漠腹地沙尘颗粒的组成研究[J].干旱区资源与环境,2017,31(11):94-99.
ZHANG Yan-wei,TANG Xiang-ling,LU Hui,et al.Atmospheric Dust Particles Collected in the Hinterland of Taklamakan Desert During the Spring,2012[J].Journal of Arid Land Resources and Environment,2017,31(11):94-99.
[21] 李 鹏,肖致美,唐 邈,等.天津典型沙尘天气过程颗粒物污染特征[J].生态与农村环境学报,2020,36(12):1532-1539.
LI Peng,XIAO Zhi-mei,TANG Miao,et al.Particulate Pollution Characteristics of Typical Sand Dust Weather in Tianjin[J].Journal of Ecology and Rural Environment,2020,36(12):1532-1539.
[22] 黄丽坤,王广智,王 琨.哈尔滨市沙尘期大气颗粒物物化特征及传输途径分析[J].中国环境科学,2014,34(8):1920-1926.
HUANG Li-kun,WANG Guang-zhi,WANG Kun.Phy-sicochemical Characteristics and Long-range Transportation of Atmospheric Particulates During a Dust Storm Episode in Harbin,China[J].China Environmental Science,2014,34(8):1920-1926.
[23] 李思思,黄正旭,王存美,等.张家口市一次沙尘天气气溶胶单颗粒理化特征和来源研究[J].生态环境学报,2017,26(3):437-444.
LI Si-si,HUANG Zheng-xu,WANG Cun-mei,et al.Chemical and Physical Characteristics and Sources of Single Particle Aerosols During a Dust Event in Zhangjiakou[J].Ecology and Environmental Scien-ces,2017,26(3):437-444.
[24] 许卫疆,车得福,蔡 宏,等.西安城郊表层黄土的粒度组成及其形态特征[J].西北大学学报(自然科学版),2004,34(2):223-227.
XU Wei-jiang,CHE De-fu,CAI Hong,et al.Grain-size Composition of Surface Layer Loess of Xi’an Ci-ty and Its Shape Character[J].Journal of Northwest University(Natural Science Edition),2004,34(2):223-227.
[25] 刘丹丹.基于Arduino平台的光散射式沙尘颗粒物浓度测量系统设计及应用[D].银川:宁夏大学,2015.
LIU Dan-dan.Design and Application of Light Scattering Dust Particle Concentration Measurement System Based on Arduino Platform[D].Yinchuan:Ning-xia University,2015.
[26] KOK J F.A Scaling Theory for the Size Distribution of Emitted Dust Aerosols Suggests Climate Models Underestimate the Size of the Global Dust Cycle[J].PNAS,2011,108(3):1016-1021.
[27] LIU M,WESTPHAL D L,WANG S G,et al.A High-resolution Numerical Study of the Asian Dust Storms of April 2001[J].Journal of Geophysical Research:Atmospheres,2003,108(D23):2002JD003178.
[28] BEHROOZ R D,MOHAMMADPOUR K,BROOMANDI P,et al.Long-term(2012-2020)PM10 Concentrations and Increasing Trends in the Sistan Basin:The Role of Levar Wind and Synoptic Meteorology[J].Atmospheric Pollution Research,2022,13(7):101460.
[29] FILONCHYK M,PETERSON M.Development,Progression,and Impact on Urban Air Quality of the Du-st Storm in Asia in March 15-18,2021[J].Urban Climate,2022,41:101080.
[30] JAAFARI J,NADDAFI K,YUNESIAN M,et al.Study of PM10,PM2.5,and PM1 Levels During Dust Storms and Local Air Pollution Events in Urban and Rural Sites in Tehran[J].Human and Ecological Risk Assessment,2018,24(2):482-493.
[31] WU C,ZHANG S,WANG G H,et al.Efficient Hete-rogeneous Formation of Ammonium Nitrate on the Saline Mineral Particle Surface in the Atmosphere of East Asia During Dust Storm Periods[J].Environmental Science & Technology,2020,54(24):15622-15630.
[32] 元天刚,陈思宇,康丽泰,等.1961~2010年中国北方沙尘源区沙尘强度时空分布特征及变化趋势[J].干旱气象,2016,34(6):927-935.
YUAN Tian-gang,CHEN Si-yu,KANG Li-tai,et al.Temporal and Spatial Distribution Characteristics and Change Trends of Dust Intensity in Dust Source Regions of Northern China During 1961-2010[J].Journal of Arid Meteorology,2016,34(6):927-935.
[33] 邓文叶,贾尔恒·阿哈提,魏明娜,等.新疆准噶尔盆地南缘一次典型沙尘污染特征分析[J].新疆环境保护,2017,39(2):1-6,17.
DENG Wen-ye,ARHATI Jia’erheng,WEI Ming-na,et al.Pollution Characteristics Analysis of a Typical Dust Event in the Southern Margin of Junggar Basin[J].Environmental Protection of Xinjiang,2017,39(2):1-6,17.
[34] HJ 1353—2024,环境空气 颗粒物来源解析 正定矩阵因子分解模型计算技术指南[S].
HJ 1353—2024,Ambient Air-source Apportionment on Particulate Matter-technical Guide on Positive Matrix Factorization Model Calculation[S].
[35] ARDON-DRYER K,KELLEY M C.Particle Size Dis-tribution and Particulate Matter Concentrations During Synoptic and Convective Dust Events in West Te-xas[J].Atmospheric Chemistry and Physics,2022,22(13):9161-9173.
[36] GINI M,MANOUSAKAS M,KARYDAS A G,et al.Mass Size Distributions,Composition and Dose Estimates of Particulate Matter in Saharan Dust Outbreaks[J].Environmental Pollution,2022,298:118768.

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Last Update: 2025-07-25